Keyword search (4,164 papers available)

"Nagapudi K" Authored Publications:

Title Authors PubMed ID
1 Resonant acoustic mixing (RAM) for efficient mechanoredox catalysis without grinding or impact media Effaty F; Gonnet L; Koenig SG; Nagapudi K; Ottenwaelder X; Frišcic T; 36546478
CHEMBIOCHEM
2 Simple, scalable mechanosynthesis of metal-organic frameworks using liquid-assisted resonant acoustic mixing (LA-RAM) Titi HM; Do JL; Howarth AJ; Nagapudi K; Frišcic T; 34094134
CHEMBIOCHEM

 

Title:Simple, scalable mechanosynthesis of metal-organic frameworks using liquid-assisted resonant acoustic mixing (LA-RAM)
Authors:Titi HMDo JLHowarth AJNagapudi KFrišcic T
Link:https://pubmed.ncbi.nlm.nih.gov/34094134/
DOI:10.1039/d0sc00333f
Publication:Chemical science
Keywords:
PMID:34094134 Category: Date Added:2021-06-07
Dept Affiliation: CHEMBIOCHEM
1 Department of Chemistry, McGill University 801 Sherbrooke St. West Montreal QC H3A 0B8 Canada tomislav.friscic@mcgill.ca.
2 Department of Chemistry and Biochemistry, Concordia University Montreal QC Canada.
3 Genentech One Dna Way South San Francisco CA 94080 USA.

Description:

We present a rapid and readily scalable methodology for the mechanosynthesis of diverse metal-organic frameworks (MOFs) in the absence of milling media typically required for other types of mechanochemical syntheses. We demonstrate the use of liquid-assisted resonant acoustic mixing (LA-RAM) methodology for the synthesis of three- and two-dimensional MOFs based on Zn(ii), Co(ii) and Cu(ii), including a mixed ligand system. Importantly, the LA-RAM approach also allowed the synthesis of the ZIF-L framework that has never been previously obtained in a mechanochemical environment, as well as its Co(ii) analogue. Straightforward scale-up from milligrams to at least 25 grams is demonstrated using the metastable framework ZIF-L as the model.





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