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The effect of step-feeding distribution ratio on high concentration perchlorate removal performance in ABR system with heterotrophic combined sulfur autotrophic process.

Author(s): Li H, Li K, Guo J, Chen Z, Han Y, Song Y, Lu C, Hou Y, Zhang D, Zhang Y

In a lab-scale anaerobic baffled reactor (ABR) with eight compartments, the heterotrophic and sulfur autotrophic processes were combined to remove perchlorate. And then, the step-feeding distribution ratio of the heterotrophic perchlorate reduction unit (HP...

Article GUID: 33485237

Acceleration mechanism of bioavailable Fe(Ⅲ) on Te(IV) bioreduction of Shewanella oneidensis MR-1: Promotion of electron generation, electron transfer and energy level.

Author(s): He Y, Guo J, Song Y, Chen Z, Lu C, Han Y, Li H, Hou Y, Zhao R

The release of highly toxic tellurite into the aquatic environment poses significant environmental risks. The acceleration mechanism and tellurium nanorods (TeNPs) characteristics with bioavailable ferric citrate (Fe(III)) were investigated in the tellurite...

Article GUID: 32853890

Exploring the biophysicochemical alteration of green alga Asterococcus superbus interactively affected by nanoparticles, triclosan and illumination.

Author(s): Xin X, Huang G, An C, Lu C, Xiong W

J Hazard Mater. 2020 May 21;398:122855 Authors: Xin X, Huang G, An C, Lu C, Xiong W

Article GUID: 32473326

Effect and ameliorative mechanisms of polyoxometalates on the denitrification under sulfonamide antibiotics stress.

Author(s): Guo H, Chen Z, Lu C, Guo J, Li H, Song Y, Han Y, Hou Y

Bioresour Technol. 2020 Feb 22;305:123073 Authors: Guo H, Chen Z, Lu C, Guo J, Li H, Song Y, Han Y, Hou Y

Article GUID: 32145698

Effect of dissolved oxygen on simultaneous removal of ammonia, nitrate and phosphorus via biological aerated filter with sulfur and pyrite as composite fillers.

Author(s): Li Y, Guo J, Li H, Song Y, Chen Z, Lu C, Han Y, Hou Y

Bioresour Technol. 2019 Oct 28;296:122340 Authors: Li Y, Guo J, Li H, Song Y, Chen Z, Lu C, Han Y, Hou Y

Article GUID: 31704601

Enhanced denitrification performance and biocatalysis mechanisms of polyoxometalates as environmentally-friendly inorganic redox mediators.

Author(s): Guo H, Chen Z, Guo J, Lu C, Song Y, Han Y, Li H, Hou Y

Bioresour Technol. 2019 Jul 16;291:121816 Authors: Guo H, Chen Z, Guo J, Lu C, Song Y, Han Y, Li H, Hou Y

Article GUID: 31344631


Title:Enhanced denitrification performance and biocatalysis mechanisms of polyoxometalates as environmentally-friendly inorganic redox mediators.
Authors:Guo HChen ZGuo JLu CSong YHan YLi HHou Y
Link:https://www.ncbi.nlm.nih.gov/pubmed/31344631?dopt=Abstract
DOI:10.1016/j.biortech.2019.121816
Category:Bioresour Technol
PMID:31344631
Dept Affiliation: ENCS
1 School of Environmental and Municipal Engineering, Tianjin Key Laboratory of Aquatic Science and Technology, Tianjin Chengjian University, Jinjing Road 26, Tianjin 300384, China.
2 Department of Building, Civil, and Environmental Engineering, Concordia University, 1455 de Maisonneuve Blvd. W, Montreal, Quebec, Canada.
3 School of Environmental and Municipal Engineering, Tianjin Key Laboratory of Aquatic Science and Technology, Tianjin Chengjian University, Jinjing Road 26, Tianjin 300384, China. Electronic address: jianbguo@163.com.
4 School of Environmental and Municipal Engineering, Tianjin Key Laboratory of Aquatic Science and Technology, Tianjin Chengjian University, Jinjing Road 26, Tianjin 300384, China. Electronic address: lucaicai2010@163.com.

Description:

Enhanced denitrification performance and biocatalysis mechanisms of polyoxometalates as environmentally-friendly inorganic redox mediators.

Bioresour Technol. 2019 Jul 16;291:121816

Authors: Guo H, Chen Z, Guo J, Lu C, Song Y, Han Y, Li H, Hou Y

Abstract

Polyoxometalates (POMs) used in chemical catalysis field were first explored their effect on the denitrification process. Experiments demonstrated that NO3--N reduction rate with 0.05?mM phosphomolybdic acid (PMo12) was approximately 3.93-fold higher than the PMo12-free system. Simultaneously, PMo12 also had positive effect on NO2--N reduction. Compared with the PMo12-free system, the solution resistance and oxidation-reduction potential were decreased, and the activation energy (Ea) was reduced by 51.84?kJ/mol. Besides, electron conductive substances in extracellular polymeric substances were stimulated by PMo12. NADH and riboflavin were enhanced to increase denitrification electron transport system activity. Higher microbial diversity and enrichment of Salmonella were observed in the PMo12-supplemented system. Based on the above analysis, the catalyzing mechanisms of PMo12 are proposed that PMo12 made it easier for electron transferring from electron donor to electron acceptor and shifted bacterial community structure. These findings may provide a promising strategy for nitrogen wastewater treatment.

PMID: 31344631 [PubMed - as supplied by publisher]